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Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2

MPS-Authors
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Kumar,  Nitesh
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Sun,  Yan
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Manna,  Kaustuv
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Süß,  Vicky
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Schmidt,  Marcus
Marcus Schmidt, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Borrmann,  Horst
Horst Borrmann, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Felser,  Claudia
Claudia Felser, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Shekhar,  Chandra
Chandra Shekhar, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Citation

Kumar, N., Sun, Y., Xu, N., Manna, K., Yao, M., Süß, V., et al. (2017). Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2. Nature Communications, 8(1): 1642, pp. 1-8. doi:10.1038/s41467-017-01758-z.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002E-560A-F
Abstract
The peculiar band structure of semimetals exhibiting Dirac and Weyl crossings can lead to spectacular electronic properties such as large mobilities accompanied by extremely high magnetoresistance. In particular, two closely neighboring Weyl points of the same chirality are protected from annihilation by structural distortions or defects, thereby significantly reducing the scattering probability between them. Here we present the electronic properties of the transition metal diphosphides, WP2 and MoP2, which are type-II Weyl semimetals with robust Weyl points by transport, angle resolved photoemission spectroscopy and first principles calculations. Our single crystals of WP2 display an extremely low residual low-temperature resistivity of 3 nΩ cm accompanied by an enormous and highly anisotropic magnetoresistance above 200 million % at 63 T and 2.5 K. We observe a large suppression of charge carrier backscattering in WP2 from transport measurements. These properties are likely a consequence of the novel Weyl fermions expressed in this compound.