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Radiative Rotational Lifetimes and State-Resolved Relative Detachment Cross Sections from Photodetachment Thermometry of Molecular Anions in a Cryogenic Storage Ring.

MPG-Autoren
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Meyer,  Christian
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Becker,  Arno
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Blaum,  Klaus
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Breitenfeldt,  Christian
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;
Institut für Physik, Ernst-Moritz-Arndt-Universität Greifswald, D-17487 Greifswald, Germany;

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George,  Sebastian
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Göck,  Jürgen
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Grieser,  Manfred
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Grussie,  Florian
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Guerin,  Elisabeth Anna
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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von Hahn,  Robert
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Herwig,  Philipp
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Krantz,  Claude
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Kreckel,  Holger
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Lion,  Jorrit
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Lohmann,  Svenja
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Mishra,  Preeti Manjari
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Novotny,  Oldrich
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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O'Connor,  Aodh
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Repnow,  Roland
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Saurabh,  Sunny
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Schwalm,  Dirk
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;
Weizmann Institute of Science, Rehovot 76100, Israel;

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Spruck,  Kaija
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;
Institut für Atom- und Molekülphysik, Justus-Liebig-Universität Gießen, D-35392 Gießen, Germany;

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Kumar,  Sunil
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Vogel,  Stephen
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Wolf,  Andreas
Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society;

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Zitation

Meyer, C., Becker, A., Blaum, K., Breitenfeldt, C., George, S., Göck, J., et al. (2017). Radiative Rotational Lifetimes and State-Resolved Relative Detachment Cross Sections from Photodetachment Thermometry of Molecular Anions in a Cryogenic Storage Ring. Physical Review Letters, 119(02): 023202. doi:10.1103/PhysRevLett.119.023202.


Zitierlink: https://hdl.handle.net/11858/00-001M-0000-002D-A0EE-6
Zusammenfassung
Photodetachment thermometry on a beam of OH in a cryogenic storage ring cooled to below 10 K is carried out using two-dimensional frequency- and time-dependent photodetachment spectroscopy over 20 min of ion storage. In equilibrium with the low-level blackbody field, we find an effective radiative temperature near 15 K with about 90% of all ions in the rotational ground state. We measure the J=1 natural lifetime (about 193 s) and determine the OH rotational transition dipole moment with 1.5% uncertainty. We also measure rotationally dependent relative near-threshold photodetachment cross sections for photodetachment thermometry.