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Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems

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Pampel,  Jonas
Tim Fellinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Fellinger,  Tim-Patrick
Tim Fellinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Antonietti,  Markus
Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Molinari,  Valerio
Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;
Valerio Molinari, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Citation

Lama, S. M. G., Pampel, J., Fellinger, T.-P., Beškoski, V. P., Slavković-Beškoski, L., Antonietti, M., et al. (2017). Efficiency of Ni Nanoparticles Supported on Hierarchical Porous Nitrogen-Doped Carbon for Hydrogenolysis of Kraft Lignin in Flow and Batch Systems. ACS Sustainable Chemistry & Engineering, 5(3), 2415-2420. doi:10.1021/acssuschemeng.6b02761.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002D-41B3-D
Abstract
Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni–C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.