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Journal Article

Thermal imaging of nanostructures by quantitative optical phase analysis

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Polleux,  Julien
Dept. New Materials and Biosystems, Max Planck Institute for Intelligent Systems, Max Planck Society;
Molecular Medicine, Max Planck Institute of Biochemistry, Max Planck Society;

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Zhu,  Min
Molecular Medicine, Max Planck Institute of Biochemistry, Max Planck Society;

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Citation

Baffou, G., Bon, P., Savatier, J., Polleux, J., Zhu, M., Merlin, M., et al. (2012). Thermal imaging of nanostructures by quantitative optical phase analysis. ACS Nano, 6(3), 2452-2458. doi:10.1021/nn2047586.


Abstract
We introduce an optical microscopy technique aimed at characterizing the heat generation arising from nanostructures, in a comprehensive and quantitative manner. Namely, the technique permits (i) mapping the temperature distribution around the source of heat, (ii) mapping the heat power density delivered by the source, and (iii) retrieving the absolute absorption cross section of light-absorbing structures. The technique is based on the measure of the thermal-induced refractive index variation of the medium surrounding the source of heat. The measurement is achieved using an association of a regular CCD camera along with a modified Hartmann diffraction grating. Such a simple association makes this technique straightforward to implement on any conventional microscope with its native broadband illumination conditions. We illustrate this technique on gold nanoparticles illuminated at their plasmonic resonance. The spatial resolution of this technique is diffraction limited, and temperature variations weaker than 1 K can be detected.