Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources

Rohringer, N.; Kimberg, V.; Weninger, C.; Sanchez-Gonzalez, A.; Lutman, A.; Maxwell, T.; Bostedt, C.; Monterro, S. Carron; Lindahl, A. O.; Ilchen, M.; Coffee, R. N.; Bozek, J. D.; Krzywinski, J.; Kierspel, T.; Mullins, T.; Kuepper, J.; Erk, B.; Rolles, D.; Muecke, O. D.; London, R. A.; Purvis, M.; Ryan, D.; Rocca, J. J.; Feifel, R.; Squibb, R.; Zhaunerchyk, V.; Sathe, C.; Agaker, M.; Mucke, M.; Nordgren, J.; Rubensson, J. E.

doi:10.1007/978-3-319-19521-6_26

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Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources

MPG-Autoren

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Rohringer, N.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Kimberg, V.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Weninger, C.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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https://link.springer.com/chapter/10.1007%2F978-3-319-19521-6_26
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Zitation

Rohringer, N., Kimberg, V., Weninger, C., Sanchez-Gonzalez, A., Lutman, A., Maxwell, T., et al. (2016). Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources. In X-Ray Lasers 2014 (pp. 201-207).

Zitierlink: https://hdl.handle.net/11858/00-001M-0000-002A-FCDA-3

Zusammenfassung

Stimulated electronic x-ray Raman scattering is the building block for several proposed x-ray pump probe techniques, that would allow the study of electron dynamics at unprecedented timescales. We present high spectral resolution data on stimulated electronic x-ray Raman scattering in a gas sample of neon using a self-amplified spontaneous emission x-ray free-electron laser. Despite the limited spectral coherence and broad bandwidth of these sources, high-resolution spectra can be obtained by statistical methods, opening the path to coherent stimulated x-ray Raman spectroscopy. An extension of these ideas to molecules and the results of a recent experiment in CO are discussed.