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Journal Article

Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy

MPS-Authors
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Kimberg,  Victor
Royal Institute of Technology, Stockholm, Sweden;
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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Mercadier,  Laurent
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons185052

Weninger,  Clemens
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;
LCLS, SLAC National Accelerator Laboratory, Menlo Park, California, USA;

/persons/resource/persons145791

Rohringer,  Nina
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

External Resource

http://dx.doi.org/10.1039/C6FD00103C
(Publisher version)

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c6fd00103c.pdf
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Citation

Kimberg, V., Sanchez-Gonzalez, A., Mercadier, L., Weninger, C., Lutman, A., Ratner, D., et al. (2016). Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy. Faraday Discussions, 194, 305-324. doi:10.1039/C6FD00103C.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002A-E792-0
Abstract
With the invention of femtosecond x-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics in the solid and liquid phase reach a new era, allowing for time-resolved x-ray diffraction and spectroscopy. To ultimately assess phase coherent electronic processes on their natural time and length scales, coherent nonlinear x-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realization of nonlinear x-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated x-ray Raman scattering in molecular gas targets.