Stimulated X-ray Raman scattering – a critical assessment of the building block 
of nonlinear X-ray spectroscopy

Kimberg, Victor; Sanchez-Gonzalez, Alvaro; Mercadier, Laurent; Weninger, Clemens; Lutman, Alberto; Ratner, Daniel; Coffee, Ryan N; Bucher, Maximilian; Mucke, Melanie; Agåker, Marcus; Såthe, Conny; Bostedt, Christoph; Nordgren, Joseph; Rubensson, Jan-Erik; Rohringer, Nina

doi:10.1039/C6FD00103C

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Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy

MPS-Authors

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Kimberg, Victor
Royal Institute of Technology, Stockholm, Sweden;
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons196618

Mercadier, Laurent
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons185052

Weninger, Clemens
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;
LCLS, SLAC National Accelerator Laboratory, Menlo Park, California, USA;

/persons/resource/persons145791

Rohringer, Nina
Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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http://dx.doi.org/10.1039/C6FD00103C
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引用

Kimberg, V., Sanchez-Gonzalez, A., Mercadier, L., Weninger, C., Lutman, A., Ratner, D., Coffee, R. N., Bucher, M., Mucke, M., Agåker, M., Såthe, C., Bostedt, C., Nordgren, J., Rubensson, J.-E., & Rohringer, N. (2016). Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy. Faraday Discussions, Advance Article. doi:10.1039/C6FD00103C.

引用: https://hdl.handle.net/11858/00-001M-0000-002A-E792-0

要旨

With the invention of femtosecond x-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics in the solid and liquid phase reach a new era, allowing for time-resolved x-ray diffraction and spectroscopy. To ultimately assess phase coherent electronic processes on their natural time and length scales, coherent nonlinear x-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realization of nonlinear x-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated x-ray Raman scattering in molecular gas targets.