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Journal Article

Two-Dimensional Spectral Interferometry using the Carrier-Envelope Phase

MPS-Authors
/persons/resource/persons37850

Ott,  Christian Reinhold
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons31009

Schönwald,  Michael
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons30920

Raith,  Philipp
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons37846

Kaldun,  Andreas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons37844

Zhang,  Yizhu
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons37848

Meyer,  Kristina
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

/persons/resource/persons30892

Pfeifer,  Thomas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

External Resource

http://m.iopscience.iop.org/1367-2630/15/7/073031
(Publisher version)

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Fulltext (public)

1108.2959.pdf
(Preprint), 711KB

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Citation

Ott, C. R., Schönwald, M., Raith, P., Kaldun, A., Zhang, Y., Meyer, K., et al. (2013). Two-Dimensional Spectral Interferometry using the Carrier-Envelope Phase. New Journal of Physics, 15(7): 073031. doi:10.1088/1367-2630/15/7/073031.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0014-5A69-3
Abstract
Two- and multi-dimensional spectroscopy is used in physics and chemistry to obtain structural and dynamical information that would otherwise be invisible by the projection into a one-dimensional data set such as a single emission or absorption spectrum. Here, we introduce a qualitatively new two-dimensional spectroscopy method by employing the carrier-envelope phase (CEP). Instead of measuring spectral vs. spectral information, the combined application of spectral interferometry and CEP control allows the measurement of otherwise inseparable temporal events on an attosecond time scale. As a specific example, we apply this general method to the case of attosecond pulse train generation, where it allows to separate contributions of three different sub-cycle electron quantum paths within one and the same laser pulse, resulting in a better physical understanding and quantification of the transition region between cutoff and plateau harmonics. The CEP-dependent separation in time between two full-cycle spaced attosecond pulses was determined to modulate by (54 +/- 16) attoseconds.