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Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways

MPG-Autoren
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Xian,  Rui
Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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Prokhorenko,  Valentyn
Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

Field,  Ryan L.
Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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Miller,  R. J. Dwayne
Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

Externe Ressourcen

http://dx.doi.org/10.1007/978-3-319-13242-6_93
(Verlagsversion)

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Zitation

Xian, R., Prokhorenko, V., Field, R. L., & Miller, R. J. D. (2015). Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways. Springer Proceedings in Physics, 162, 382-385.


Zitierlink: https://hdl.handle.net/11858/00-001M-0000-0024-BE47-B
Zusammenfassung
We perform closed- and open-loop coherent control experiments of the photodissociation of triiodide (I3−) in ethanol using shaped UV pulses. In the regime where the relative diiodide (I2−) yield is excitation-independent, we observe a symmetrical second-order chirp dependence of the I2− yield, and that the I2− production can be controlled within 40 % by varying the second-order chirp of the pump pulse. We show that additional pathways involving higher-lying potential energy surfaces are viable means to explain such observations.