Attosecond Correlated Dynamics of Two Electrons Passing through a Transition 
State

Camus, Nicolas; Fischer, B.; Kremer, M.; Sharma, V.; Rudenko, A.; Bergues, Boris; Kübel, Matthias; Johnson, Nora G.; Kling, Matthias F.; Pfeifer, T.; Ullrich, J.; Moshammer, R.

doi:10.1103/PhysRevLett.108.073003

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Attosecond Correlated Dynamics of Two Electrons Passing through a Transition State

MPS-Authors

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Camus, Nicolas
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Fischer, B.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Kremer, M.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Sharma, V.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Rudenko, A.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Bergues, Boris
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

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Kübel, Matthias
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

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Johnson, Nora G.
Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

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Kling, Matthias F.
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

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Pfeifer, T.
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Ullrich, J.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Moshammer, R.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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http://link.aps.org/doi/10.1103/PhysRevLett.108.073003
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Citation

Camus, N., Fischer, B., Kremer, M., Sharma, V., Rudenko, A., Bergues, B., et al. (2012). Attosecond Correlated Dynamics of Two Electrons Passing through a Transition State. Physical Review Letters, 108(7): 073003, pp. 1-5. doi:10.1103/PhysRevLett.108.073003.

Cite as: https://hdl.handle.net/11858/00-001M-0000-0014-B453-C

Abstract

he strong-field induced decay of a doubly excited, transient Coulomb complex Ar^**→Ar²⁺+2e^- is explored by tracing correlated two-electron emission in nonsequential double ionization of Ar as a function of the carrier-envelope phase. Using <6 fs pulses, electron emission is essentially confined to one optical cycle. Classical model calculations support that the intermediate Coulomb complex has lost memory of its formation dynamics and allows for a consistent, though model-dependent definition of “emission time,” empowering us to trace transition-state two-electron decay dynamics with sub-fs resolution. We find a most likely emission time difference of ∼200±100 as.