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Journal Article

Attosecond Correlated Dynamics of Two Electrons Passing through a Transition State

MPS-Authors
http://pubman.mpdl.mpg.de/cone/persons/resource/persons37832

Camus,  Nicolas
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30471

Fischer,  B.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30723

Kremer,  M.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31041

Sharma,  V.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30960

Rudenko,  A.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60415

Bergues,  Boris
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60648

Kübel,  Matthias
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60590

Johnson,  Nora G.
Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60619

Kling,  Matthias F.
Attosecond Imaging, Laboratory for Attosecond Physics, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30892

Pfeifer,  T.
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31125

Ullrich,  J.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30822

Moshammer,  R.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Citation

Camus, N., Fischer, B., Kremer, M., Sharma, V., Rudenko, A., Bergues, B., et al. (2012). Attosecond Correlated Dynamics of Two Electrons Passing through a Transition State. Physical Review Letters, 108(7): 073003, pp. 1-5. doi:10.1103/PhysRevLett.108.073003.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0014-B453-C
Abstract
he strong-field induced decay of a doubly excited, transient Coulomb complex Ar**→Ar2++2e- is explored by tracing correlated two-electron emission in nonsequential double ionization of Ar as a function of the carrier-envelope phase. Using <6  fs pulses, electron emission is essentially confined to one optical cycle. Classical model calculations support that the intermediate Coulomb complex has lost memory of its formation dynamics and allows for a consistent, though model-dependent definition of “emission time,” empowering us to trace transition-state two-electron decay dynamics with sub-fs resolution. We find a most likely emission time difference of ∼200±100 as.