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Direct coupling of alcohols to form esters and amides with evolution of H2 using in situ formed ruthenium catalysts

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Prechtl,  Martin H. G.
Institut für Technische und Makromolekulare Chemie, Rheinisch-Westfälische Technische Hochschule Aachen;
Service Department Leitner (Technical Labs), Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Wobser,  Kathrin
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Theyssen,  Nils
Service Department Theyssen (Technical Labs), Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Leitner,  Walter
Institut für Technische und Makromolekulare Chemie, Rheinisch-Westfälische Technische Hochschule Aachen;
Service Department Leitner (Technical Labs), Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Prechtl, M. H. G., Wobser, K., Theyssen, N., Ben-David, Y., Milstein, D., & Leitner, W. (2012). Direct coupling of alcohols to form esters and amides with evolution of H2 using in situ formed ruthenium catalysts. Catalysis Science & Technology, 2(12), 2039-2042. doi:10.1039/c2cy20429k.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0014-A2AE-2
Abstract
A simple approach for the catalytic conversion of primary alcohols into their corresponding esters and amides, with evolution of H2 gas using in situ formed ruthenium PNP- and PNN-pincer catalysts, is presented. The evaluation showed conversions for the esterification with turnover numbers as high as 4300, and 4400 for the amidation.