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Trends in the Binding Strength of Surface Species on Nanoparticles: How Does the Adsorption Energy Scale with the Particle Size?

MPS-Authors
http://pubman.mpdl.mpg.de/cone/persons/resource/persons21952

Peter,  Matthias
Chemical Physics, Fritz Haber Institute, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons21516

Flores Camacho,  Jose Manuel
Chemical Physics, Fritz Haber Institute, Max Planck Society;
Instituto de Investigación en Comunicación Óptica-UASLP;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons32621

Adamovski,  Sergey
Chemical Physics, Fritz Haber Institute, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons32692

Dostert,  Karl-Heinz
Chemical Physics, Fritz Haber Institute, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons36554

O'Brien,  Casey
Chemical Physics, Fritz Haber Institute, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons22062

Schauermann,  Swetlana
Chemical Physics, Fritz Haber Institute, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons21524

Freund,  Hans-Joachim
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Citation

Peter, M., Flores Camacho, J. M., Adamovski, S., Ono, L. K., Dostert, K.-H., O'Brien, C., et al. (2013). Trends in the Binding Strength of Surface Species on Nanoparticles: How Does the Adsorption Energy Scale with the Particle Size? Angewandte Chemie International Edition, 52(19), 5175-5179. doi:10.1002/anie.201209476.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0014-61D5-C
Abstract
Thumbnail image of graphical abstract The binding energy of oxygen on Pd nanoparticles was measured by a direct calorimetric method as a function of the particle size. The reduced dimensionality of the Pd substrate results in two counteracting trends: an increase of the Pd[BOND]O binding strength due to a change of the local configuration of the adsorption site and a strong decrease of the Pd[BOND]O bonding due to the reduction of the cluster size.