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Journal Article

Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2

MPS-Authors
http://pubman.mpdl.mpg.de/cone/persons/resource/persons30470

Fischer,  Andreas
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31069

Sperl,  Alexander Georg
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons37942

Cörlin,  Philipp
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31009

Schönwald,  Michael
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30947

Rietz,  Helga
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30892

Pfeifer,  Thomas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31125

Ullrich,  Joachim
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
Physikalisch-Technische Bundesanstalt, Bundesallee 100, 38116 Braunschweig, Germany;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons31033

Senftleben,  Arne
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30822

Moshammer,  Robert
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Citation

Fischer, A., Sperl, A. G., Cörlin, P., Schönwald, M., Rietz, H., Palacios, A., et al. (2013). Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2. Physical Review Letters, 110(21): 213002, pp. 1-5. doi:10.1103/PhysRevLett.110.213002.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0014-18E3-1
Abstract
Dissociative single ionization of H2 induced by extreme ultraviolet photons from an attosecond pulse train has been studied in a kinematically complete experiment. Depending on the electron kinetic energy and the alignment of the molecule with respect to the laser polarization axis, we observe pronounced asymmetries in the relative emission directions of the photoelectron and the H+ ion. The energy-dependent asymmetry pattern is explained by a semiclassical model and further validated by fully quantum mechanical calculations, both in very good agreement with the experiment.