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Journal Article

Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2

MPS-Authors
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Fischer,  Andreas
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Sperl,  Alexander Georg
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Cörlin,  Philipp
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Schönwald,  Michael
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Rietz,  Helga
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Pfeifer,  Thomas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Ullrich,  Joachim
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
Physikalisch-Technische Bundesanstalt, Bundesallee 100, 38116 Braunschweig, Germany;

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Senftleben,  Arne
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Moshammer,  Robert
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

External Resource

http://prl.aps.org/abstract/PRL/v110/i21/e213002
(Publisher version)

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Citation

Fischer, A., Sperl, A. G., Cörlin, P., Schönwald, M., Rietz, H., Palacios, A., et al. (2013). Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2. Physical Review Letters, 110(21): 213002, pp. 1-5. doi:10.1103/PhysRevLett.110.213002.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0014-18E3-1
Abstract
Dissociative single ionization of H2 induced by extreme ultraviolet photons from an attosecond pulse train has been studied in a kinematically complete experiment. Depending on the electron kinetic energy and the alignment of the molecule with respect to the laser polarization axis, we observe pronounced asymmetries in the relative emission directions of the photoelectron and the H+ ion. The energy-dependent asymmetry pattern is explained by a semiclassical model and further validated by fully quantum mechanical calculations, both in very good agreement with the experiment.