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Fractional high-order harmonic combs and energy tuning by attosecond-precision split-spectrum pulse control

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Raith,  Philipp
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Ott,  Christian
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Kaldun,  Andreas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Laux,  Martin
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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Pfeifer,  Thomas
Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society;

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引用

Raith, P., Ott, C., Anderson, C. P., Kaldun, A., Meyer, K., Laux, M., Zhang, Y., & Pfeifer, T. (2012). Fractional high-order harmonic combs and energy tuning by attosecond-precision split-spectrum pulse control. Applied Physics Letters, 100(12):, pp. 1-5. doi:10.1063/1.3693615.


引用: https://hdl.handle.net/11858/00-001M-0000-000E-8B2F-4
要旨
We experimentally control high-order harmonic generation by applying a versatile few-cycle pulse-shape control method: splitting up a single broadband continuous laser spectrum into two sections and applying sub-femtosecond relative time delays. For certain time delays, fractional high-harmonic combs (noninteger harmonics) are generated which we find to result from the controlled interference of two attosecond pulse trains. We also observe time-delay-dependent energy-tunability of the high-order harmonics for an asymmetrically split spectrum consisting of a strong and a weak component. The tuning mechanism is quantitatively understood by the controlled modulation of the instantaneous driver frequency at the peak of the shaped laser pulse.