Modeling Zeolites with Metal-Supported Two-Dimensional Aluminosilicate Films

Boscoboinik, Anibal; Yu, Xin; Yang, Bing; Fischer, Frank Daniel; Włodarczyk, Radosław; Sierka, Marek; Shaikhutdinov, Shamil Kamilovich; Sauer, Joachim; Freund, Hans-Joachim

doi:10.1002/anie.201201319

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Modeling Zeolites with Metal-Supported Two-Dimensional Aluminosilicate Films

MPS-Authors

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Boscoboinik, Anibal
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Yu, Xin
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Yang, Bing
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Shaikhutdinov, Shamil Kamilovich
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Freund, Hans-Joachim
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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引用

Boscoboinik, A., Yu, X., Yang, B., Fischer, F. D., Włodarczyk, R., Sierka, M., Shaikhutdinov, S. K., Sauer, J., & Freund, H.-J. (2012). Modeling Zeolites with Metal-Supported Two-Dimensional Aluminosilicate Films. Angewandte Chemie International Edition, 51(24), 6005-6008. doi:10.1002/anie.201201319.

引用: https://hdl.handle.net/11858/00-001M-0000-0010-241E-7

要旨

Flat pore models: Thin, well-defined aluminosilicate films with tetrahedral [SiO_4/2] and [AlO_4/2⁻] building blocks that are weakly bound to an underlying metal support contain highly acidic bridging OH species, which exhibit H–D exchange (see picture; Si yellow, O red, Al gray, C black, H white). These films are a model system for surface-science studies of the inner walls of zeolite pores.