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Journal Article

Intramolecular Redox-Triggered C-H Functionalization

MPS-Authors
http://pubman.mpdl.mpg.de/cone/persons/resource/persons58657

Jurberg,  Igor Dias
Research Group Maulide, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons58879

Peng,  Bo
Research Group Maulide, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons59122

Wöstefeld,  Eckhard
Research Group Maulide, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons58381

Wasserloos,  Maximilian
Research Group Maulide, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons58809

Maulide,  Nuno
Research Group Maulide, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Jurberg, I. D., Peng, B., Wöstefeld, E., Wasserloos, M., & Maulide, N. (2012). Intramolecular Redox-Triggered C-H Functionalization. Angewandte Chemie International Edition: a journal of the Gesellschaft Deutscher Chemiker, 51(8), 1950-1953. doi:10.1002/anie.201108639.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0010-20BD-1
Abstract
Sacrifice for the team: A one-pot method achieves remote functionalization at the α-position of an amine moiety through the sacrificial reduction of a neighboring group. The process takes advantage of an intramolecular redox reaction, thereby avoiding the need for any external oxidants. This method was applied to a concise five-step total synthesis of indolizidine 167B.