de.mpg.escidoc.pubman.appbase.FacesBean
English
 
Help Guide Disclaimer Contact us Login
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT

Released

Journal Article

Optimal control of ground-state dynamics in polymers

MPS-Authors
http://pubman.mpdl.mpg.de/cone/persons/resource/persons60961

Zeidler,  D.
Laser Chemistry, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60492

Frey,  S.
Laser Chemistry, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60949

Wohlleben,  W.
Laser Chemistry, Max Planck Institute of Quantum Optics, Max Planck Society;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons60712

Motzkus,  M.
Laser Chemistry, Max Planck Institute of Quantum Optics, Max Planck Society;

Locator
There are no locators available
Fulltext (public)
There are no public fulltexts available
Supplementary Material (public)
There is no public supplementary material available
Citation

Zeidler, D., Frey, S., Wohlleben, W., Motzkus, M., Busch, F., Chen, T., et al. (2002). Optimal control of ground-state dynamics in polymers. Journal of Chemical Physics, 116(12), 5231-5235. Retrieved from http://ojps.aip.org/getabs/servlet/GetabsServlet?prog=normal&id=JCPSA6000116000012005231000001&idtype=cvips&gifs=Yes.


Cite as: http://hdl.handle.net/11858/00-001M-0000-000F-C237-2
Abstract
Coherent control of the vibrational dynamics in crystalline polydiacetylene is demonstrated by tailoring the Stokes pulse of a coherent anti-Stokes Raman scattering (CARS) setup in a feedback-controlled self-learning loop. The feedback signal is derived from the spectral distribution of the CARS signal. Controlled excitation of one mode and simultaneous extinction of all other modes with high efficiency is demonstrated. In addition, the relative phases of the three normal modes have been controlled allowing excitations of local modes and suggesting the possibility of ground state reaction control. (C) 2002 American Institute of Physics.