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Free-Electron Lasers: New Avenues in Molecular Physics and Photochemistry

MPG-Autoren
http://pubman.mpdl.mpg.de/cone/persons/resource/persons31125

Ullrich,  Joachim H.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
Max Planck Advanced Study Group, Center for Free-Electron Laser Science, D-22607 Hamburg, Germany;
Physikalisch-Technische Bundesanstalt, D-38116 Braunschweig, Germany;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30960

Rudenko,  Artem
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
Max Planck Advanced Study Group, Center for Free-Electron Laser Science, D-22607 Hamburg, Germany;

http://pubman.mpdl.mpg.de/cone/persons/resource/persons30822

Moshammer,  Robert
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Zitation

Ullrich, J. H., Rudenko, A., & Moshammer, R. (2012). Free-Electron Lasers: New Avenues in Molecular Physics and Photochemistry. In Annual Review of Physical Chemistry (pp. 635-660). Palo Alto: Annual Reviews Inc. doi:10.1146/annurev-physchem-032511-143720.


Zitierlink: http://hdl.handle.net/11858/00-001M-0000-000F-A42C-4
Zusammenfassung
Free-electron lasers are fourth-generation light sources that deliver extremely intense (>10−12 −photons per pulse), ultrashort ( 10−14 s = 10 fs) light pulses at up to kilohertz repetition rates with unprecedented coherence properties and span a broad wavelength regime from soft ( 10 eV) to hard X-ray energies ( 15 keV). They thus enable a whole suite of novel experiments in molecular physics and chemistry: Inspecting radiation-induced reactions in cold molecular ions provides unprecedented insight into the photochemistry of interstellar clouds and upper planetary atmospheres; double core-hole photoelectron spectroscopy offers enhanced sensitivity for chemical analysis; the dynamics of highly excited molecular states, pumped by vacuum ultraviolet pulses, can be inspected; and vacuum ultraviolet or X-ray probe pulses generally hold the promise to trace chemical reactions along an entire reaction coordinate with atomic spatial and temporal resolution. This review intends to provide a first overview on upcoming possibilities, emerging technologies, pioneering results, and future perspectives in this exciting field.