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  Role of intraband transitions in photocarrier generation

Sato, S., Lucchini, M., Volkov, M., Schlaepfer, F., Gallmann, L., Keller, U., et al. (2018). Role of intraband transitions in photocarrier generation. Physical Review B, 98(3): 035202. doi:10.1103/PhysRevB.98.035202.

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PhysRevB.98.035202.pdf (Verlagsversion), 934KB
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PhysRevB.98.035202.pdf
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2018
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© American Physical Society

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externe Referenz:
https://dx.doi.org/10.1103/PhysRevB.98.035202 (Verlagsversion)
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https://arxiv.org/abs/1804.03678 (Preprint)
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 Urheber:
Sato, S.1, 2, Autor           
Lucchini, M.3, Autor
Volkov, M.4, Autor
Schlaepfer, F.4, Autor
Gallmann, L.4, Autor
Keller, U.4, Autor
Rubio, A.1, 2, 5, Autor           
Affiliations:
1Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
2Center for Free-Electron Laser Science, ou_persistent22              
3Department of Physics, Politecnico di Milano, ou_persistent22              
4Department of Physics, ETH Zürich, ou_persistent22              
5Center for Computational Quantum Physics, The Flatiron Institute, ou_persistent22              

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 Zusammenfassung: We theoretically investigate the role of intraband transitions in laser-induced carrier generation for different photon energy regimes: (i) strongly off resonant, (ii) multiphoton resonant, and (iii) resonant conditions. Based on the analysis for the strongly off resonant and multiphoton resonant cases, we find that intraband transitions strongly enhance photocarrier generation in both multiphoton absorption and tunneling excitation regimes, and thus, they are indispensable for describing the nonlinear photocarrier generation processes. Furthermore, we find that intraband transitions enhance photocarrier generation even in the resonant condition, opening additional multiphoton excitation channels once the laser irradiation becomes sufficiently strong. The above findings suggest a potential for efficient control of photocarrier generation via multicolor laser pulses through optimization of the contributions from intraband transitions.

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Sprache(n): eng - English
 Datum: 2018-06-042018-04-102018-07-052018-07-05
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1103/PhysRevB.98.035202
arXiv: 1804.03678
 Art des Abschluß: -

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Projektname : This work was supported by the European Research Council (Grant No. ERC-2015-AdG-694097), Grupos Consolidados (IT578-13), European Union’s H2020 program under Grant Agreement No. 676580 (NOMAD), and the National Center of Competence in Research Molecular Ultrafast Science and Technology (NCCR MUST) funded by the Swiss National Science Foundation. S.A.S. gratefully acknowledges the fellowship from the Alexander von Humboldt Foundation.
Grant ID : 676580
Förderprogramm : Horizon 2020 (H2020)
Förderorganisation : European Commission (EC)

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Titel: Physical Review B
  Kurztitel : Phys. Rev. B
Genre der Quelle: Zeitschrift
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Affiliations:
Ort, Verlag, Ausgabe: Woodbury, NY : American Physical Society
Seiten: - Band / Heft: 98 (3) Artikelnummer: 035202 Start- / Endseite: - Identifikator: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008