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  Poly(ionic liquid)-mediated morphogenesis of bismuth sulfide with a tunable band gap and enhanced electrocatalytic properties

Gao, M.-R., Yu, S.-H., Yuan, J., Zhang, W., & Antonietti, M. (2016). Poly(ionic liquid)-mediated morphogenesis of bismuth sulfide with a tunable band gap and enhanced electrocatalytic properties. Angewandte Chemie International Edition, 55(41), 12812-12816. doi:10.1002/anie.201607221.

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 Creators:
Gao, Min-Rui1, Author
Yu, Shu-Hong, Author
Yuan, Jiayin1, Author           
Zhang, Weiyi1, Author           
Antonietti, Markus2, Author           
Affiliations:
1Jiayin Yuan, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863318              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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Free keywords: bismuth sulfide; inorganic crystals; morphogenesis; poly(ionic liquid)s; polymer-controlled crystallization Anorganische Kristalle, Bismutsulfid, Morphogenese, Polymere ionische Flüssigkeiten, Polymerkontrollierte Kristallisation
 Abstract: Conventional polymer additives have a substantial impact on synthetic inorganic chemistry, but critical shortcomings remain; for example, low solubility in organic solvents and potential thermodynamic aggregates. Poly(ionic liquid)s have now been used as efficient additives that enable a high level control of bismuth sulfide crystals with significant size and morphological diversities. The bismuth sulfides exhibit tunable band structure as a result of the quantum size effects. Moreover, poly(ionic liquid)s are able to couple with as-synthesized bismuth sulfides chemically and endow a modified surface electronic structure, which allows resultant products to possess outstanding electrocatalytic performance for water oxidation, although its commercial counterpart is catalytically inert.

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Language(s): eng - English
 Dates: 2016-09-152016
 Publication Status: Issued
 Pages: -
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Title: Angewandte Chemie International Edition
  Abbreviation : Angew. Chem., Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 55 (41) Sequence Number: - Start / End Page: 12812 - 12816 Identifier: ISSN: 1433-7851

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Title: Angewandte Chemie
  Abbreviation : Angew. Chem.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 128 (41) Sequence Number: - Start / End Page: 13004 - 13008 Identifier: ISSN: 0044-8249