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  Tracing nuclear-wave-packet dynamics in singly and doubly charged states of N2 and O2 with XUV-pump–XUV-probe experiments

Magrakvelidze, M., Herrwerth, O., Jiang, Y. H., Rudenko, A., Kurka, M., Foucar, L., et al. (2012). Tracing nuclear-wave-packet dynamics in singly and doubly charged states of N2 and O2 with XUV-pump–XUV-probe experiments. Physical Review A, 86(1): 013415, pp. 1-11. doi:10.1103/PhysRevA.86.013415.

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Magrakvelidze, M., Author
Herrwerth , O., Author
Jiang, Y. H., Author
Rudenko , A., Author
Kurka, M., Author
Foucar, Lutz1, Author           
Kühnel, K. U., Author
Kübel, M., Author
Johnson, Nora G., Author
Schröter, C. D., Author
Düsterer, S., Author
Treusch, R., Author
Lezius, M., Author
Ben-Itzhak, I., Author
Moshammer, R., Author
Ullrich , J., Author
Kling, M. F., Author
Thumm, and U., Author
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: We traced the femtosecond nuclear-wave-packet dynamics in ionic states of oxygen and nitrogen diatomic molecules employing 38-eV XUV-pump–XUV-probe experiments at the free-electron laser in Hamburg (FLASH). The nuclear dynamics is monitored via the detection of coincident ionic fragments using a reaction microscope and a split-mirror setup to generate the pump and probe pulses. By comparing measured kinetic-energy-release spectra with classical and quantum-mechanical simulations, we identified electronic states of the molecular ions that are populated by ionization of the neutral molecule. For specific fragment charge states, this comparison allows us to assess the relevance of specific dissociation paths

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Language(s): eng - English
 Dates: 2012-03-082012-07-182012-07-18
 Publication Status: Issued
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 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevA.86.013415
Other: 7972
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Title: Physical Review A
  Other : Phys. Rev. A
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: - Volume / Issue: 86 (1) Sequence Number: 013415 Start / End Page: 1 - 11 Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2