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  Dynamics of hollow atom formation in intense x-ray pulses probed by partial covariance mapping

Frasinski, L. J., Zhaunerchyk, V., Mucke, M., Squibb, R. J., Siano, M., Eland, J. H. D., et al. (2013). Dynamics of hollow atom formation in intense x-ray pulses probed by partial covariance mapping. Physical Review Letters, 111(7): 073002, pp. 1-5. doi: 10.1103/PhysRevLett.111.073002.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0019-9095-0 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0019-9096-E
Genre: Journal Article

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PhysRevLett_111_2013_073002_1.pdf (Any fulltext), 877KB
 
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 Creators:
Frasinski, L. J., Author
Zhaunerchyk, V., Author
Mucke, M., Author
Squibb, R. J., Author
Siano, M., Author
Eland, J. H. D., Author
Linusson, P., Author
Meulen, P. v.d., Author
Salén, P., Author
Thomas, R. D., Author
Larsson, M., Author
Foucar, Lutz1, Author           
Ullrich, J., Author
Motomura, K., Author
Mondal, S., Author
Ueda, K., Author
Osipov, T., Author
Fang, L., Author
Murphy, B. F., Author
Berrah, N., Author
Bostedt, C., AuthorBozek, J. D., AuthorSchorb, S., AuthorMesserschmidt, M., AuthorGlownia, J. M., AuthorCryan, J. P., AuthorCoffee, R. N., AuthorTakahashi, O., AuthorWada, S., AuthorPiancastelli, M. N., AuthorRichter, R., AuthorPrince, K. C., AuthorFeifel, R., Author more..
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: When exposed to ultraintense x-radiation sources such as free electron lasers (FELs) the innermost electronic shell can efficiently be emptied, creating a transient hollow atom or molecule. Understanding the femtosecond dynamics of such systems is fundamental to achieving atomic resolution in flash diffraction imaging of noncrystallized complex biological samples. We demonstrate the capacity of a correlation method called “partial covariance mapping” to probe the electron dynamics of neon atoms exposed to intense 8 fs pulses of 1062 eV photons. A complete picture of ionization processes competing in hollow atom formation and decay is visualized with unprecedented ease and the map reveals hitherto unobserved nonlinear sequences of photoionization and Auger events. The technique is particularly well suited to the high counting rate inherent in FEL experiments.

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Language(s): eng - English
 Dates: 2013-04-102013-08-132013-08-13
 Publication Status: Issued
 Pages: -
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 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.111.073002
Other: 7957
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Pages: - Volume / Issue: 111 (7) Sequence Number: 073002 Start / End Page: 1 - 5 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1