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  An oscillating liquid-gas reaction with periodic evaporation : nonlinear analysis and experimental results

Zeyer, K. P., Mangold, M., Obertopp, T., & Gilles, E. D. (1999). An oscillating liquid-gas reaction with periodic evaporation: nonlinear analysis and experimental results. Chemical Engineering Science, 54(21), 4845-4851. doi:10.1016/S0009-2509(99)00203-1.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0013-A287-3 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0027-AC69-6
Genre: Journal Article

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 Creators:
Zeyer, K. P.1, Author              
Mangold, M.1, Author              
Obertopp, T.2, Author
Gilles, E. D.2, 3, Author              
Affiliations:
1Process Synthesis and Process Dynamics, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, escidoc:1738153              
2Universität Stuttgart, escidoc:persistent22              
3Systems Biology, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, escidoc:1738155              

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 Abstract: In this work we present theoretical and experimental studies of a laboratory scale continuous flow stirred tank reactor (CSTR) in which theiron-(III)-nitrate catalyzed oxidation of ethanol with hydrogen peroxide to ethanal and acetic acid takes place. This reaction displays temperature and concentration oscillations when it is performed in a CSTR. A liquid phase model is known in the literature derived from a more detailed mechanism. This model predicts the location of stationary solutions and bifurcations well, but the calculated reactor temperatures are high above the boiling point of the reaction mixture under certain conditions. Therefore, two different gas/liquid models were developed and compared with the experimental results. © Copyright 2004 Elsevier Science B.V., Amsterdam. All rights reserved. [accessed 2014 March 31st]

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Language(s): eng - English
 Dates: 1999
 Publication Status: Published in print
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 Rev. Method: -
 Identifiers: eDoc: 111976
DOI: 10.1016/S0009-2509(99)00203-1
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Title: Chemical Engineering Science
Source Genre: Journal
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Pages: - Volume / Issue: 54 (21) Sequence Number: - Start / End Page: 4845 - 4851 Identifier: -