Steady-state and forced periodic operation of solid electrolyte membrane 
reactors for selective oxidation of n-butane to maleic anhydride

Munder, Barbara; Rihko-Struckmann, Liisa; Sundmacher, Kai

doi:10.1016/j.ces.2007.01.042

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Steady-state and forced periodic operation of solid electrolyte membrane reactors for selective oxidation of n-butane to maleic anhydride

Munder, B., Rihko-Struckmann, L., & Sundmacher, K. (2007). Steady-state and forced periodic operation of solid electrolyte membrane reactors for selective oxidation of n-butane to maleic anhydride. Chemical Engineering Science, 62(18-20 ), 5663-5668. doi:10.1016/j.ces.2007.01.042.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0013-9919-A Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0027-8334-4

Genre: Journal Article

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Creators:
Munder, Barbara¹, Author
Rihko-Struckmann, Liisa¹, Author
Sundmacher, Kai^{1, 2}, Author

Affiliations:
1Process Systems Engineering, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, ou_1738151
2Otto-von-Guericke-Universität Magdeburg, External Organizations, ou_1738156

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Abstract: Experimental results obtained with a bilayer-solid electrolyte membrane reactor (bilayer-SEMR) are analysed based on a 1D+1D reactor model and attainable yields in steady-state and forced-periodic operation modes are determined. Optimal steady-state operation conditions are predicted in the range of high Damköhler numbers and oxidizing conditions. Forced-periodic operation of bilayer-SEMRs, which is easily established via the electric current, leads to a significant selectivity enhancement, but has to be critically rated with respect to energy expenses needed under electrochemical-oxygen-pumping conditions. copyright 2007 Elsevier Ltd. All rights reserved. [accessed February 8th 2013]

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Language(s): eng - English

Dates: Date issued: 2007

Publication Status: Issued

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Rev. Type: Peer

Identifiers: eDoc: 281003
Other: 12/07
DOI: 10.1016/j.ces.2007.01.042

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Title: Chemical Engineering Science

Source Genre: Journal

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Pages: - Volume / Issue: 62 (18-20 ) Sequence Number: - Start / End Page: 5663 - 5668 Identifier: -