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  Nonlinear-optical processes in the near-resonant two-photon excitation of xenon by femtosecond KrF-excimer-laser pulses

Tünnermann, A., Mossavi, K., & Wellegehausen, B. (1992). Nonlinear-optical processes in the near-resonant two-photon excitation of xenon by femtosecond KrF-excimer-laser pulses. Physical Review A, 46(5), 2707-2717. doi:10.1103/PhysRevA.46.2707.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0013-5C83-4 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0013-5C84-2
Genre: Journal Article

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PhyRevA46-2707.pdf (Publisher version), 2MB
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Tünnermann, Andreas1, Author
Mossavi, Kasem2, Author              
Wellegehausen, B., Author
Affiliations:
1External Organizations, escidoc:persistent13              
2Laser Interferometry & Gravitational Wave Astronomy, AEI-Hannover, MPI for Gravitational Physics, Max Planck Society, escidoc:24010              

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 Abstract: The nonlinear response of xenon gas due to a near-resonant two-photon excitation at the 5p6 1S0→6p[1/2]0 transition with a femtosecond KrF-excimer-laser system is investigated for the intensity range 1010–1015 W/cm2. Stimulated hyper-Raman scattering and amplified spontaneous emission of atomic xenon are observed at wavelengths around 823 and 828 nm. These emissions are superimposed by four-wave parametric-oscillation processes leading to strong ultrashort continuum radiation in the visible and near-infrared (650–850 nm), uv (185–400 nm), and vacuum ultraviolet (147–155 nm) spectral ranges with output powers up to 100 MW. From difference-frequency-mixing experiments microscopic nonlinear susceptibilities in the range of ‖χ(3)‖=10-48 to 10-50 m5/V2 have been determined, which are in good agreement with calculations.

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 Dates: 1992-07
 Publication Status: Published in print
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 Identifiers: eDoc: 376553
DOI: 10.1103/PhysRevA.46.2707
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Title: Physical Review A
Source Genre: Journal
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Pages: - Volume / Issue: 46 (5) Sequence Number: - Start / End Page: 2707 - 2717 Identifier: ISSN: 1094-1622