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  Femtosecond x-ray photoelectron diffraction on gas-phase dibromobenzene molecules

Rolles, D., Boll, R., Adolph, M., Aquila, A., Bostedt, C., Bozek, J. D., et al. (2014). Femtosecond x-ray photoelectron diffraction on gas-phase dibromobenzene molecules. Journal of Physics B, 47(12): 124035. doi:10.1088/0953-4075/47/12/124035.

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https://dx.doi.org/10.1088/0953-4075/47/12/124035 (Verlagsversion)
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 Urheber:
Rolles, Daniel1, 2, 3, Autor           
Boll , R1, 2, 4, Autor
Adolph, M5, Autor
Aquila, A6, 7, Autor
Bostedt, C8, Autor
Bozek, J D8, Autor
Chapman, H N6, 9, 10, Autor
Coffee, R8, Autor
Coppola, N6, 7, Autor
Decleva, P11, Autor
Delmas, T6, Autor
Epp, S. W.1, 4, 12, Autor           
Erk, B1, 2, 4, Autor
Filsinger, Frank13, 14, Autor           
Foucar, L1, 3, Autor
Gumprecht, L6, Autor
Hömke, A1, 2, 4, Autor
Gorkhover, T5, Autor
Holmegaard, L6, 15, Autor
Johnsson, P16, Autor
Kaiser, Ch4, AutorKrasniqi, F1, 3, 17, Autor           Kühnel, K-U4, AutorMaurer, J15, AutorMesserschmidt, M8, AutorMoshammer, R4, AutorQuevedo, Wilson18, 19, Autor           Rajkovic, Ivan18, 20, Autor           Rouzée, A21, 22, AutorRudek, B1, 2, 4, 23, AutorSchlichting, Ilme1, 3, Autor           Schmidt, C1, 2, 4, AutorSchorb, S5, 8, AutorSchröter, C D4, AutorSchulz, J6, 7, AutorStapelfeldt, H15, AutorStener, M11, AutorStern, S6, 9, AutorTechert, Simone2, 18, 24, Autor           Thøgersen, J15, AutorVrakking, M J J21, 22, AutorRudenko, A1, 4, 25, AutorKüpper, Jochen1, 6, 9, 10, 13, Autor           Ullrich, J1, 4, 23, Autor mehr..
Affiliations:
1Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany , ou_persistent22              
2Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany , ou_persistent22              
3Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              
4Max Planck Institute for Nuclear Physics, 69117 Heidelberg, Germany , ou_persistent22              
5Technische Universität Berlin, 10623 Berlin, Germany , ou_persistent22              
6Center for Free-Electron Laser Science, DESY, 22607 Hamburg, Germany , ou_persistent22              
7European X-ray Free-Electron Laser (XFEL) GmbH, 22761 Hamburg, Germany , ou_persistent22              
8SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA, ou_persistent22              
9Department of Physics, University of Hamburg, 22761 Hamburg, Germany , ou_persistent22              
10The Hamburg Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
11Dipartimento di Scienze Chimiche e Farmaceutiche, Universita di Trieste, 34127 Trieste, Italy , ou_persistent22              
12Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, Luruper Chaussee 149, Geb. 99 (CFEL), 22761 Hamburg, DE, ou_1938288              
13Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
14Bruker AXS GmbH, 76187 Karlsruhe, Germany, ou_persistent22              
15Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
16Department of Physics, Lund University, 22100 Lund, Sweden, ou_persistent22              
17Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, Luruper Chaussee 149, Geb. 99 (CFEL), 22761 Hamburg, DE, ou_1938293              
18Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for biophysical chemistry, Max Planck Society, ou_578564              
19Helmholtz-Zentrum Berlin, 12489 Berlin, Germany, ou_persistent22              
20Paul-Scherrer-Institut, 5232 Villingen, Switzerland, ou_persistent22              
21Max-Born-Institut, 12489 Berlin, Germany, ou_persistent22              
22FOM-Institute AMOLF, 1098 XG Amsterdam, The Netherlands , ou_persistent22              
23Physikalisch-Technische Bundesanstalt (PTB), 38116 Braunschweig, Germany , ou_persistent22              
24Institute of X-ray Physics, Göttingen University, 37077 Göttingen, Germany , ou_persistent22              
25JR MacDonald Laboratory, Kansas State University, Manhattan, KS 66506, USA , ou_persistent22              

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 Zusammenfassung: We present time-resolved femtosecond photoelectron momentum images and angular distributions of dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules measured in a near-infrared pump, soft-x-ray probe experiment performed at an x-ray free-electron laser. The observed alignment dependence of the bromine 2p photoelectron angular distributions is compared to density functional theory calculations and interpreted in terms of photoelectron diffraction. While no clear time-dependent effects are observed in the angular distribution of the Br(2p) photoelectrons, other, low-energy electrons show a pronounced dependence on the time delay between the near-infrared laser and the x-ray pulse.

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Sprache(n): eng - English
 Datum: 2014-01-022014-03-252014-06-102014-06-28
 Publikationsstatus: Erschienen
 Seiten: 12
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1088/0953-4075/47/12/124035
 Art des Abschluß: -

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Titel: Journal of Physics B
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Bristol, UK : IOP Pub.
Seiten: - Band / Heft: 47 (12) Artikelnummer: 124035 Start- / Endseite: - Identifikator: ISSN: 0953-4075
CoNE: https://pure.mpg.de/cone/journals/resource/954928494403