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  Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S. W., Cryle, M., et al. (2013). Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging. Journal of Physics B: Atomic, Molecular and Optical Physics, 46(16): 164031. doi:10.1088/0953-4075/46/16/164031.

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Datensatz-Permalink: http://hdl.handle.net/11858/00-001M-0000-0014-B4A9-E Versions-Permalink: http://hdl.handle.net/11858/00-001M-0000-0014-B4AA-C
Genre: Zeitschriftenartikel

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 Urheber:
Erk, Benjamin1, 2, 3, Autor              
Rolles, Daniel2, 3, 4, Autor              
Foucar, Lutz3, 4, Autor              
Rudek, Benedikt1, 2, 3, Autor              
Epp, S. W.1, 3, Autor              
Cryle, Max4, Autor              
Bostedt, C5, Autor
Schorb, S5, 6, Autor
Bozek, J5, Autor
Rouzee, A7, Autor
Hundertmark, A7, Autor
Marchenko, T8, Autor
Simon, M8, Autor
Filsinger, Frank9, Autor              
Christensen, L10, Autor
De, S11, 12, Autor
Trippel, S13, Autor
Küpper, Jochen13, 14, 15, Autor              
Stapelfeldt, H11, Autor
Wada, S5, 16, Autor
Ueda, K17, AutorSwiggers, M5, AutorMesserschmidt, M5, AutorSchröter, Claus Dieter1, Autor              Moshammer, Robert1, 3, Autor              Schlichting, I.3, 4, Autor              Ullrich, Joachim H.1, 3, 18, Autor              Rudenko, Artem1, 2, 19, Autor               mehr..
Affiliations:
1Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society, escidoc:904547              
2Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany , escidoc:persistent22              
3Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany , escidoc:persistent22              
4Max Planck Institute for Medical Research, escidoc:1125545              
5Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, United States , escidoc:persistent22              
6 Institut für Optik und Atomare Physik, Technische Universität Berlin, 10623 Berlin, Germany , escidoc:persistent22              
7Max-Born-Institut, 12489 Berlin, Germany , escidoc:persistent22              
8Laboratoire de Chimie Physique-Matière et Rayonnement, CNRS, UPMC, 75231 Paris, France , escidoc:persistent22              
9Molecular Physics, Fritz Haber Institute, Max Planck Society, escidoc:634545              
10Department of Physics and Astronomy, Aarhus University, Aarhus, Denmark , escidoc:persistent22              
11Department of Chemistry, Aarhus University, 8000 Aarhus, Denmark, escidoc:persistent22              
12Saha Institute of Nuclear Physics, 700064 Kolkata, India , escidoc:persistent22              
13Center for Free-Electron Laser Science (CFEL), DESY, 22607 Hamburg, Germany , escidoc:persistent22              
14Department of Physics, University of Hamburg, escidoc:persistent22              
15Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, escidoc:persistent22              
16Department of Physical Science, Hiroshima University, 739-8526 Higashi-Hiroshima, Japan , escidoc:persistent22              
17IMRAM, Tohoku University, 980-8577 Sendai, Japan , escidoc:persistent22              
18Physikalisch-Technische Bundesanstalt, 38116 Braunschweig, Germany , escidoc:persistent22              
19J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, United States , escidoc:persistent22              

Inhalt

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Schlagwörter: -
 Zusammenfassung: The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH3SeH) and ethylselenol (C2H5SeH), by intense (>1017 W cm-2) 5 fs x-ray pulses with photon energies of 1.7 and 2 keV has been studied by means of coincident ion momentum spectroscopy. Measuring charge states and ion kinetic energies, we find signatures of charge redistribution within the molecular environment. Furthermore, by analyzing fragment ion angular correlations, we can determine the laboratory-frame orientation of individual molecules and thus investigate the fragmentation dynamics in the molecular frame. This allows distinguishing protons originating from different molecular sites along with identifying the reaction channels that lead to their emission.

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Sprache(n): eng - Englisch
 Datum: 2013-08-19
 Publikationsstatus: Online publiziert
 Seiten: 12
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1088/0953-4075/46/16/164031
 Art des Abschluß: -

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Quelle 1

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Titel: Journal of Physics B: Atomic, Molecular and Optical Physics
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Bristol, UK : IOP Pub.
Seiten: - Band / Heft: 46 (16) Artikelnummer: 164031 Start- / Endseite: - Identifikator: ISSN: 0953-4075
CoNE: http://pubman.mpdl.mpg.de/cone/journals/resource/954928494403