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  Continuous-Flow Hydrogenation of Carbon Dioxide to Pure Formic Acid using an Integrated scCO2 Process with Immobilized Catalyst and Base

Wesselbaum, S., Hintermair, U., & Leitner, W. (2012). Continuous-Flow Hydrogenation of Carbon Dioxide to Pure Formic Acid using an Integrated scCO2 Process with Immobilized Catalyst and Base. Angewandte Chemie International Edition: a journal of the Gesellschaft Deutscher Chemiker, 51(34), 8585-8588. doi:10.1002/anie.201203185.

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anie_201203185_sm_miscellaneous_information.pdf (Supplementary material), 2MB
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anie_201203185_sm_miscellaneous_information.pdf
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Supporting Information
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application/pdf / [MD5]
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Copyright Date:
2012
Copyright Info:
Wiley-VCH, 69451 Weinheim, Germany
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 Creators:
Wesselbaum, Sebastian1, 2, Author
Hintermair, Ulrich1, 3, Author
Leitner, Walter1, 4, Author           
Affiliations:
1Institut für Technische Chemie, RWT Aachen University, Worringerweg 1, 52056 Aachen, ou_persistent22              
2Research Group of Nanoscale Spin Imaging, MPI for Biophysical Chemistry, Max Planck Society, Am Faßberg 11, 37077 Göttingen, DE, ou_1113579              
3Department of Chemistry, Yale University, 225 Prospect Stret, New Haven, CT 06520, USA, ou_persistent22              
4Service Department Leitner (Technical Labs), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445626              

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Free keywords: carbon dioxide fixation formic acid homogeneous catalysis hydrogenation supercritical fluids
 Abstract: Dual role for CO2: Pure formic acid can be obtained continuously by hydrogenation of CO2 in a single processing unit (see scheme). An immobilized ruthenium organometallic catalyst and a nonvolatile base in an ionic liquid (IL) are combined with supercritical CO2 as both reactant and extractive phase.

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Language(s): eng - English
 Dates: 2012-05-312012-04-252012-07-132012-08-20
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201203185
 Degree: -

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Title: Angewandte Chemie International Edition : a journal of the Gesellschaft Deutscher Chemiker
Source Genre: Journal
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Publ. Info: Weinheim/Bergstr. : Verlag Chemie
Pages: 4 Volume / Issue: 51 (34) Sequence Number: - Start / End Page: 8585 - 8588 Identifier: ISSN: 0570-0833
CoNE: https://pure.mpg.de/cone/journals/resource/110984073528720