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  Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S., Cryle, M. J., et al. (2013). Ultrafast Charge Rearrangement and Nuclear Dynamics upon Inner-Shell Multiple Ionization of Small Polyatomic Molecules. Physical Review Letters, 110(5): 053003. doi:10.1103/PhysRevLett.110.053003.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-A0B6-F Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-A0B7-D
Genre: Journal Article

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PhysRevLett.110.053003.pdf (Publisher version), 673KB
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 Creators:
Erk, Benjamin1, 2, Author           
Rolles, D.1, 3, 4, Author           
Foucar, L.1, 3, Author           
Rudek, Benedikt1, 2, 4, Author           
Epp, Sascha2, Author           
Cryle, M. J.3, Author           
Bostedt, C.5, Author           
Schorb, S.5, 6, Author           
Bozek, J.5, Author
Rouzee, A.7, Author
Hundertmark, A.7, Author
Marchenko, T.8, Author           
Simon, M.8, Author
Filsinger, Frank9, Author           
Christensen, L10, Author           
De, S.11, 12, Author           
Trippel, S.13, Author           
Küpper, Jochen13, 14, Author           
Stapelfeldt, H.11, Author
Wada, S5, 15, Author           
Ueda, K.16, Author           Swiggers, M.5, AuthorMesserschmidt, M.5, AuthorSchroeter, C.D.2, Author           Moshammer, Robert2, Author           Schlichting, I.1, 3, Author           Joachim, U.1, 2, 17, Author           Rudenko, A.1, 2, 18, Author            more..
Affiliations:
1Max Planck Advanced Study Group (ASG) at CFEL, 22761 Hamburg, Germany, ou_persistent22              
2Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society, ou_904547              
3Max Planck Institute for Medical Research, ou_1125545              
4DESY, 22607 Hamburg, Germany, ou_persistent22              
5Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
6Institut für Optik und Atomare Physik, Technische Universität Berlin, 10623 Berlin, Germany, ou_persistent22              
7Max Born Institute, 12489 Berlin, Germany, ou_persistent22              
8Laboratoire de Chimie Physique-Matière et Rayonnement, CNRS and UPMC, 75231 Paris, France, ou_persistent22              
9Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
10Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
11Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
12Saha Institute of Nuclear Physics, 700064 Kolkata, India, ou_persistent22              
13Center for Free-Electron Laser Science (CFEL), DESY, 22607 Hamburg, Germany, ou_persistent22              
14Department of Physics, University of Hamburg, ou_persistent22              
15Department of Physical Science, Hiroshima University, 739-8526 Higashi-Hiroshima, Japan, ou_persistent22              
16IMRAM, Tohoku University, 980-8577 Sendai, Japan, ou_persistent22              
17Physikalisch-Technische Bundesanstalt, 38116 Braunschweig, Germany, ou_persistent22              
18J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA, ou_persistent22              

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 Abstract: Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017  W/cm2) 5 fs x-ray pulses (ℏω=2  keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner-shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization.

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Language(s): eng - English
 Dates: 2012-10-022013-01-302013-01-30
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: ISI: 000314231800005
DOI: 10.1103/PhysRevLett.110.053003
 Degree: -

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Title: Physical Review Letters
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 110 (5) Sequence Number: 053003 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1