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  Trends in the Binding Strength of Surface Species on Nanoparticles: How Does the Adsorption Energy Scale with the Particle Size?

Peter, M., Flores Camacho, J. M., Adamovski, S., Ono, L. K., Dostert, K.-H., O'Brien, C., et al. (2013). Trends in the Binding Strength of Surface Species on Nanoparticles: How Does the Adsorption Energy Scale with the Particle Size? Angewandte Chemie International Edition, 52(19), 5175-5179. doi:10.1002/anie.201209476.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-61D5-C Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-7655-7
Genre: Journal Article

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 Creators:
Peter, Matthias1, Author           
Flores Camacho, Jose Manuel1, 2, Author           
Adamovski, Sergey1, Author           
Ono, Luis K.3, Author
Dostert, Karl-Heinz1, Author           
O'Brien, Casey1, Author           
Roldan Cuenya, Beatriz3, Author
Schauermann, Swetlana1, Author           
Freund, Hans-Joachim1, Author           
Affiliations:
1Chemical Physics, Fritz Haber Institute, Max Planck Society, ou_24022              
2Instituto de Investigación en Comunicación Óptica-UASLP, Av. Karakorum 1470, 78210 San Luis Potosi (Mexico), ou_persistent22              
3University of Central Florida, Department of Physics, 4000 Central Florida Boulevard, Orlando, FL 32816 (USA), ou_persistent22              

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Free keywords: adsorption calorimetry; binding strength; metal nanoparticles; oxygen; palladium
 Abstract: Thumbnail image of graphical abstract The binding energy of oxygen on Pd nanoparticles was measured by a direct calorimetric method as a function of the particle size. The reduced dimensionality of the Pd substrate results in two counteracting trends: an increase of the Pd[BOND]O binding strength due to a change of the local configuration of the adsorption site and a strong decrease of the Pd[BOND]O bonding due to the reduction of the cluster size.

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Language(s): eng - English
 Dates: 2012-11-272013-04-052013-05-03
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201209476
 Degree: -

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Title: Angewandte Chemie International Edition
  Other : Angewandte Chemie - International Edition
  Abbreviation : Angew. Chem. Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH Verlag GmbH & Co. KGaA
Pages: - Volume / Issue: 52 (19) Sequence Number: - Start / End Page: 5175 - 5179 Identifier: CoNE: https://pure.mpg.de/cone/journals/resource/201310171