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  Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2

Fischer, A., Sperl, A. G., Cörlin, P., Schönwald, M., Rietz, H., Palacios, A., et al. (2013). Electron Localization Involving Doubly Excited States in Broadband Extreme Ultraviolet Ionization of H2. Physical Review Letters, 110(21): 213002, pp. 1-5. doi:10.1103/PhysRevLett.110.213002.

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Fischer, Andreas1, Author           
Sperl, Alexander Georg1, Author           
Cörlin, Philipp1, Author           
Schönwald, Michael2, Author           
Rietz, Helga1, Author           
Palacios, Alicia3, Author
González-Castrillo, Alberto3, Author
Martín, Fernando3, 4, Author
Pfeifer, Thomas2, Author           
Ullrich, Joachim1, 5, Author           
Senftleben, Arne1, Author           
Moshammer, Robert1, Author           
Affiliations:
1Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society, ou_904547              
2Thomas Pfeifer - Independent Junior Research Group, Junior Research Groups, MPI for Nuclear Physics, Max Planck Society, ou_907555              
3Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain, ou_persistent22              
4Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA-Nanociencia), Cantoblanco, 28049 Madrid, Spain, ou_persistent22              
5Physikalisch-Technische Bundesanstalt, Bundesallee 100, 38116 Braunschweig, Germany, ou_persistent22              

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 Abstract: Dissociative single ionization of H2 induced by extreme ultraviolet photons from an attosecond pulse train has been studied in a kinematically complete experiment. Depending on the electron kinetic energy and the alignment of the molecule with respect to the laser polarization axis, we observe pronounced asymmetries in the relative emission directions of the photoelectron and the H+ ion. The energy-dependent asymmetry pattern is explained by a semiclassical model and further validated by fully quantum mechanical calculations, both in very good agreement with the experiment.

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Language(s): eng - English
 Dates: 2013-05-20
 Publication Status: Published online
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.110.213002
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Title: Physical Review Letters
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 110 (21) Sequence Number: 213002 Start / End Page: 1 - 5 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1