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  Investigation of solid/vapor interfaces using ambient pressure X-ray photoelectron spectroscopy

Starr, D. E., Liu, Z., Hävecker, M., Knop-Gericke, A., & Bluhm, H. (2013). Investigation of solid/vapor interfaces using ambient pressure X-ray photoelectron spectroscopy. Chemical Society Reviews, 42(13), 5833-5857. doi:10.1039/c3cs60057b.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0013-FAF7-C Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0018-FB66-5
Genre: Journal Article

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 Creators:
Starr, D. E.1, Author
Liu, Z.2, Author
Hävecker, Michael3, 4, Author           
Knop-Gericke, Axel3, Author           
Bluhm, H.5, Author
Affiliations:
1Solar Energy Research, Energy Materials In-situ Laboratory (EMIL), Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, D-12489 Berlin, Germany , ou_persistent22              
2Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, USA, ou_persistent22              
3Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
4Catalysis for Energy, Group E-GKAT, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, D-12489 Berlin, Germany, ou_persistent22              
5Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, USA, ou_persistent22              

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 Abstract: Heterogeneous chemical reactions at vapor/solid interfaces play an important role in many processes in the environment and technology. Ambient pressure X-ray photoelectron spectroscopy (APXPS) is a valuable tool to investigate the elemental composition and chemical specificity of surfaces and adsorbates on the molecular scale at pressures of up to 130 mbar. In this review we summarize the historical development of APXPS since its introduction over forty years ago, discuss different approaches to minimize scattering of electrons by gas molecules, and give a comprehensive overview about the experimental systems (vapor/solid interfaces) that have been studied so far. We also present several examples for the application of APXPS to environmental science, heterogeneous catalysis, and electrochemistry.

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Language(s): eng - English
 Dates: 2013-02-082013-04-192013-07-07
 Publication Status: Issued
 Pages: 25
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/c3cs60057b
 Degree: -

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Title: Chemical Society Reviews
  Other : Chem. Soc. Rev.
Source Genre: Journal
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Publ. Info: London : Royal Society of Chemistry, etc.
Pages: - Volume / Issue: 42 (13) Sequence Number: - Start / End Page: 5833 - 5857 Identifier: ISSN: 0306-0012
CoNE: https://pure.mpg.de/cone/journals/resource/110992357259182