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  The Intimate Relationship between Bulk Electronic Conductivity and Selectivity in the Catalytic Oxidation of n-Butane

Eichelbaum, M., Hävecker, M., Heine, C., Karpov, A., Dobner, C.-K., Rosowski, F., et al. (2012). The Intimate Relationship between Bulk Electronic Conductivity and Selectivity in the Catalytic Oxidation of n-Butane. Angewandte Chemie International Edition: a journal of the Gesellschaft Deutscher Chemiker, 51(25), 6246-6250. doi:10.1002/anie.201201866.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-000F-9DF0-1 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0013-FB16-D
Genre: Journal Article

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2012
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 Creators:
Eichelbaum, Maik1, Author           
Hävecker, Michael1, 2, Author           
Heine, Christian1, Author           
Karpov, Andrey3, Author
Dobner, Cornelia-Katharina3, Author
Rosowski, Frank3, Author
Trunschke, Annette1, Author           
Schlögl, Robert1, Author           
Affiliations:
1Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
2Helmholtz-Zentrum Berlin fuer Materialien und Energy GmbH, Division Solar Energy Research, Elektronenspeicherring BESSY II, ou_persistent22              
3Chemicals Research and Engineering BASF SE, Carl- Bosch-Straße 38, 67056 Ludwigshafen (Deutschland), ou_persistent22              

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Free keywords: electrical conductivity; heterogeneous catalysis; in situ spectroscopy; oxidation
 Abstract: Don’t touch! Without electrode contacts, but contact-free with microwaves in a resonant cavity the electronic conductivity of a VPO powder catalyst could be measured under the reaction conditions of the selective oxidation of n-butane to maleic anhydride. As a result, a linear correlation between conductivity and formation rate of maleic anhydride was observed.

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Language(s): eng - English
 Dates: 2012-04-262012-05-082012
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201201866
 Degree: -

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Title: Angewandte Chemie International Edition : a journal of the Gesellschaft Deutscher Chemiker
Source Genre: Journal
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Publ. Info: Weinheim/Bergstr. : Verlag Chemie
Pages: - Volume / Issue: 51 (25) Sequence Number: - Start / End Page: 6246 - 6250 Identifier: ISSN: 0570-0833
CoNE: https://pure.mpg.de/cone/journals/resource/110984073528720