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  Total Synthesis of Amphidinolide F

Valot, G., Regens, C. S., O'Malley, D. P., Godineau, E., Takikawa, H., & Fürstner, A. (2013). Total Synthesis of Amphidinolide F. Angewandte Chemie International Edition, 52(36), 9534-9538. doi:10.1002/anie.201301700.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-A3B5-8 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0024-C252-1
Genre: Journal Article

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anie_201301700_sm_miscellaneous_information.pdf (Supplementary material), 7MB
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https://hdl.handle.net/11858/00-001M-0000-0014-A3B7-4
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anie_201301700_sm_miscellaneous_information.pdf
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Supporting Information
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Copyright Date:
2013
Copyright Info:
Wiley-VCH, 69451 Weinheim, Germany
License:
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 Creators:
Valot, Gaëlle1, Author           
Regens, Christopher S.1, Author           
O'Malley, Daniel P.1, Author           
Godineau, Edouard1, Author           
Takikawa, Hiroshi1, Author           
Fürstner, Alois1, Author           
Affiliations:
1Research Department Fürstner, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445584              

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Free keywords: alkyne metathesis; molybdenum; natural products; platinum; total synthesis
 Abstract: Orchestrated yet nonconsonant: The challenge posed by the “umpoled” 1,4-dioxygenation pattern characteristic for the polyketide frame of amphidinolide F was mastered by a late-stage ring-closing alkyne metathesis followed by a directed transannular hydration under the aegis of a carbophilic π-acid catalyst. This concordant strategy enabled a concise total synthesis of this enticing marine natural product.

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Language(s): eng - English
 Dates: 2013-04-222013-09-02
 Publication Status: Issued
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201301700
 Degree: -

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Title: Angewandte Chemie International Edition
  Other : Angew. Chem., Int. Ed.
  Abbreviation : Angew. Chem. Int. Ed
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH Verlag GmbH & Co. KGaA
Pages: 8 Volume / Issue: 52 (36) Sequence Number: - Start / End Page: 9534 - 9538 Identifier: CoNE: https://pure.mpg.de/cone/journals/resource/1433-7851
ISSN: 1433-7851